Hybrid nanostructures based on protein-assembly driven by carbohydrate-protein interactions
Final Report Abstract
Synthesis of functional hybrid materials via soft-template method has attracted increasing at-tentions as it is feasible for the formation of various complex ordered nanostructures (e.g. hi-erarchical porous structure), thus providing large space for the control over desired architec-tures as well as functionalities. Compared to the hard template, soft template is ease of tem-plate removal via simple solvent extraction or calcination. Our project focuses on the synthesis of novel functional composite materials with desired complex structures and functionalities us-ing soft-template approach. Specifically, three different soft templates have been applied for the synthesis of versatile composite particles within our study, including glycopeptide biomol-ecules, self-assembled block copolymer particles, and poly(ionic liquid) nanovesicles. Related fundamental aspects, such as template preparation, composite material fabrication, and their application in catalysis, have been well addressed in the study. Possible applications of the obtained composite particles as efficient catalysts have been studied in two representative reactions, i.e. reduction of 4-nitrophenol and CO2 electroreduction.
Publications
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Cryo-Electron microscopy for the study of self-assembled poly(ionic liquid) nanoparticles and protein supramolecular structures. Colloid and Polymer Science, 298(7), 707-717.
Kochovski, Zdravko; Chen, Guosong; Yuan, Jiayin & Lu, Yan
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Fabrication of Pascal‐triangle Lattice of Proteins by Inducing Ligand Strategy. Angewandte Chemie International Edition, 59(24), 9617-9623.
Liu, Rongying; Kochovski, Zdravko; Li, Long; Yin, Yue‐wen; Yang, Jing; Yang, Guang; Tao, Guoqing; Xu, Anqiu; Zhang, Ensong; Ding, Hong‐ming; Lu, Yan; Chen, Guosong & Jiang, Ming
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Synthetic advances of internally nanostructured polymer particles: From and beyond block copolymer. Nano Select, 1(6), 639-658.
Pan, Xuefeng; Mei, Shilin; Lu, Yan & Yuan, Jiayin
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A Comprehensive Landscape for Fibril Association Behaviors Encoded Synergistically by Saccharides and Peptides. Journal of the American Chemical Society, 143(17), 6622-6633.
Liu, Rongying; Zhang, Ran; Li, Long; Kochovski, Zdravko; Yao, Lintong; Nieh, Mu-Ping; Lu, Yan; Shi, Tongfei & Chen, Guosong
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Colloidal dispersion of poly(ionic liquid)/Cu composite particles for protective surface coating against SAR‐CoV‐2. Nano Select, 3(1), 227-232.
Khorsand, Kheirabad Atefeh; Pan, Xuefeng; Long, Siwen; Kochovski, Zdravko; Zhou, Shiqi; Lu, Yan; McInerney, Gerald & Yuan, Jiayin
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Construction of Active Protein Materials: Manipulation on Morphology of Salmon Calcitonin Assemblies with Enhanced Bone Regeneration Effect. Advanced Materials, 34(45).
Wu, Libin; Cheng, Liang; Yang, Jing; Yan, Yufei; Zhang, Ensong; Kochovski, Zdravko; Li, Long; Wang, Zhen; Deng, Lianfu; Lu, Yan; Besenius, Pol; Cui, Wenguo & Chen, Guosong
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Template synthesis of dual-functional porous MoS2nanoparticles with photothermal conversion and catalytic properties. Nanoscale, 14(18), 6888-6901.
Pan, Xuefeng; Sarhan, Radwan M.; Kochovski, Zdravko; Chen, Guosong; Taubert, Andreas; Mei, Shilin & Lu, Yan
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Evolution of Protein Assemblies Driven by the Switching of Interplay Mode. ACS Nano, 17(3), 2245-2256.
Liu, Rongying; Li, Long; Chen, Shuyu; Yang, Zhiwei; Kochovski, Zdravko; Mei, Shilin; Lu, Yan; Zhang, Lei & Chen, Guosong
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Multi-functionalized carbon nanotubes towards green fabrication of heterogeneous catalyst platforms with enhanced catalytic properties under NIR light irradiation. Nanoscale, 15(38), 15749-15760.
Pan, Xuefeng; Liu, Rongying; Yu, Zhilong; Haas, Benedikt; Kochovski, Zdravko; Cao, Sijia; Sarhan, Radwan M.; Chen, Guosong & Lu, Yan
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Poly(ionic liquid) nanovesicles via polymerization induced self-assembly and their stabilization of Cu nanoparticles for tailored CO2 electroreduction. Journal of Colloid and Interface Science, 637, 408-420.
Pan, Xuefeng; Kochovski, Zdravko; Wang, Yong-Lei; Sarhan, Radwan M.; Härk, Eneli; Gupta, Siddharth; Stojkovikj, Sasho; El-Nagar, Gumaa A.; Mayer, Matthew T.; Schürmann, Robin; Deumer, Jérôme; Gollwitzer, Christian; Yuan, Jiayin & Lu, Yan
