Stehende Dichtewellen in epitaktischen nicht-kommensurablen Molekülschichten
Zusammenfassung der Projektergebnisse
The project aimed at the demonstration of the assumed universal role static distortion waves (SDWs) play in the structure formation of organic adsorbates which exhibit non-commensurate epitaxy. To that end, several different molecule–substrate combinations were investigated structurally by means of low-temperature STM and distortion-corrected LEED. While many promising structures were indeed found, a direct proof for the presence of SDWs could not be achieved. A theoretical, machine-learning-based method was developed that allows to simulate systems with sufficiently large unit cells to capture the formation of SDWs. This method was successfully applied to naphthalene on Cu(111) and provides new insights into the impact of SDWs on the friction at inorganic/organic interfaces.
Projektbezogene Publikationen (Auswahl)
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High Potassium Concentrations Nested in Epitaxial Monolayers of a Flexible Lander-Type Molecule on Ag(111). The Journal of Physical Chemistry C, 124(7), 4114-4127.
Otto, Felix; Kirchhuebel, Tino; Baby, Anu; Sojka, Falko; Fratesi, Guido; Fritz, Torsten & Forker, Roman
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Hybridization vs decoupling: influence of an h-BN interlayer on the physical properties of a lander-type molecule on Ni(111). Beilstein Journal of Nanotechnology, 11, 1168-1177.
Schaal, Maximilian; Aihara, Takumi; Gruenewald, Marco; Otto, Felix; Domke, Jari; Forker, Roman; Yoshida, Hiroyuki & Fritz, Torsten
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Role of Initial and Final States in Molecular Spectroscopies: Example of Tetraphenyldibenzoperiflanthene (DBP) on Graphite. The Journal of Physical Chemistry C, 124(36), 19622-19638.
Kirchhuebel, Tino; Kera, Satoshi; Munakata, Toshiaki; Ueno, Nobuo; Shiraishi, Ryo; Yamaguchi, Takuma; Yonezawa, Keiichirou; Ueba, Takahiro; Bussolotti, Fabio; Yang, Jinpeng; Yamada, Takashi; Mori, Ryosuke; Kunieda, Shogo; Huempfner, Tobias; Gruenewald, Marco; Forker, Roman & Fritz, Torsten
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An alternative route towards the fabrication of 2D blue phosphorene. Journal of Physics: Condensed Matter, 33(48), 485002.
Schaal, M.; Picker, J.; Otto, F.; Gruenewald, M.; Forker, R. & Fritz, T.
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Nonintuitive Surface Self-Assembly of Functionalized Molecules on Ag(111). ACS Nano, 15(4), 6723-6734.
Jeindl, Andreas; Domke, Jari; Hörmann, Lukas; Sojka, Falko; Forker, Roman; Fritz, Torsten & Hofmann, Oliver T.
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Blue phosphorene on Au(111) as a decoupling layer for organic epitaxially grown films. Physical Review Materials, 6(1).
Gruenewald, Marco; Schaal, Maximilian; Karadzhov, Iliyan; Brill, Lorenz; Domke, Jari; Grimm, Philip; Otto, Felix; Picker, Julian; Simon, Paul M.; Tamm, Hendrik; Fritz, Torsten & Forker, Roman
