Modellierung photoschaltbarer Hybridmaterialien aus organischen Molekülen und Graphen
Physikalische Chemie von Festkörpern und Oberflächen, Materialcharakterisierung
Zusammenfassung der Projektergebnisse
This project was initially granted in July 2015 as part of an ERA-NET project with the universities of Mons, Strasbourg, and Montpellier. The KIT funding was 36 months E13. While at KIT we were early able to recruit Dr. Velimir Meded to work on this project, recruitment of our principal collaboration partner, the group of Prof. Samori in Strasbourg was delayed to the lack of availability of suitable personnel. Just when Prof. Samori was able to hire a postdoc to work on this project, Dr. Meded was forced to leave KIT, because our request to grant him a permanent position was denied for reasons that I still fail to understand. His work resulted in publications #1 & #2 enumerated below. We subsequently hired sequentially 2 students, Gianni Procida and Emanuela Carrieri, to work on this project but both failed to make sufficient progress towards the goals of the project and the Ph.D. as a whole, so both left the group. Their work is discussed briefly in the report discussed below, but because Prof. Samori had meanwhile published the experimental results this work has not been published to date. In order to continue very promising ongoing work on the subject area of the proposal, we applied for a cost-neutral extension of the project, which was granted by the EU and the DFG. The work performed in the extension period, which resulted in publications #3 to #8, is discussed in detail below. Overall, the 36 PM of postdoc funding resulted in 7 internationally visible journals, including 1 publication in ACS Nano and 1 publication in ACS Applied Materials and Interfaces, 2 publications in Advanced Materials, and 2 in Angew. Chemie. Intl. Edition in which this project provided modeling and simulation.
Projektbezogene Publikationen (Auswahl)
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Superexchange Charge Transport in Loaded Metal Organic Frameworks. ACS Nano 2016, 10 (7), 7085–7093
Neumann, T.; Liu, J.; Wächter, T.; Friederich, P.; Symalla, F.; Welle, A.; Mugnaini, V.; Meded, V.; Zharnikov, M.; Wöll, C.; Wenzel, W.
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Switching the Proton Conduction in Nanoporous, Crystalline Materials by Light. Advanced Materials 2018, 30 (8), 1706551
Müller, K.; Helfferich, J.; Zhao, F.; Verma, R.; Kanj, A. B.; Meded, V.; Bléger, D.; Wenzel, W.; Heinke, L.
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Conductance Photoswitching of Metal–Organic Frameworks with Embedded Spiropyran. Angewandte Chemie International Edition 2019, 58 (4), 1193–1197
Garg, S.; Schwartz, H.; Kozlowska, M.; Kanj, A. B.; Müller, K.; Wenzel, W.; Ruschewitz, U.; Heinke, L.
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Photoconductivity in Metal-Organic Framework (MOF) Thin Films. Angew. Chem.-Int. Edit. 2019, 58 (28), 9590–9595
Liu, X.; Kozlowska, M.; Okkali, T.; Wagner, D.; Higashino, T.; Brenner-Weifss, G.; Marschner, S. M.; Fu, Z.; Zhang, Q.; Imahori, H.; Braese, S.; Wenzel, W.; Woell, C.; Heinke, L.
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Halogenated Terephthalic Acid “Antenna Effects” in Lanthanide-SURMOF Thin Films,ACS Appl. Mater. Interfaces 2020, 12, 46, 52166–52174
Jaciara C. C. Santos, Yohanes Pramudya, Marjan Krstić, Dong-Hui Chen, Beatrice Lilli Neumeier, Claus Feldmann, Wolfgang Wenzel, and Engelbert Redel
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Contact Spacing Controls the On-Current for All-Carbon Field Effect Transistors. Commun Phys 2021, 4 (1), 1–12
Özdemir, A. D.; Barua, P.; Pyatkov, F.; Hennrich, F.; Chen, Y.; Wenzel, W.; Krupke, R.; Fediai, A.
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Modeling the Layer-by-Layer Growth of HKUST-1 Metal-Organic Framework Thin Films. Nanomaterials 2021, 11 (7)
Zhang, Q.; Pramudya, Y.; Wenzel, W.; Wöll, C.
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Sensing Molecules with Metal–Organic Framework Functionalized Graphene Transistors. Advanced Materials 2021, 33 (43), 2103316
Kumar, S.; Pramudya, Y.; Müller, K.; Chandresh, A.; Dehm, S.; Heidrich, S.; Fediai, A.; Parmar, D.; Perera, D.; Rommel, M.; Heinke, L.; Wenzel, W.; Wöll, C.; Krupke, R.
